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ID: ALA1154654

Journal: Bioorg Med Chem Lett

Title: Design and synthesis of novel histone deacetylase inhibitor derived from nuclear localization signal peptide.

Authors: Canzoneri JC, Chen PC, Oyelere AK.

Abstract: We describe herein the synthesis and characterization of a new class of histone deacetylase (HDAC) inhibitors derived from conjugation of a suberoylanilide hydroxamic acid-like aliphatic-hydroxamate pharmacophore to a nuclear localization signal peptide. We found that these conjugates inhibited the histone deacetylase activities of HDACs 1, 2, 6, and 8 in a manner similar to suberoylanilide hydroxamic acid (SAHA). Notably, compound 7b showed a threefold improvement in HDAC 1/2 inhibition, a threefold increase in HDAC 6 selectivity and a twofold increase in HDAC 8 selectivity when compared to SAHA.

CiteXplore: 19854643

DOI: 10.1016/j.bmcl.2009.10.028