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ID: ALA1821576

Journal: Eur J Med Chem

Title: Synthesis and antitumour activity of β-hydroxyisovalerylshikonin analogues.

Authors: Rao Z, Liu X, Zhou W, Yi J, Li SS.

Abstract: A series of novel β-hydroxyisovalerylshikonin analogues bearing oxygen-containing substituents at the side-chain hydroxyl of shikonin were designed and synthesized. The cytotoxicities of these compounds were evaluated in vitro against multi-drug resistant (MDR) cell lines DU-145 and HeLa. Most compounds exhibited significant inhibitory activity on both cell lines. The structure-activity relationship showed the analogues with ether substituents displayed the most potent antitumour activity and selective cytotoxicity towards DU-145. Among the compounds with ether substituents, increasing the steric hindrance in the carbon bearing β-hydroxyl or replace the β-hydroxyl with acetoxy or methoxy would lead to the decline of cytotoxicity.

CiteXplore: 21689869

DOI: 10.1016/j.ejmech.2011.05.065